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A review on emulsification via microfluidic processes

Yichen Liu, Yongli Li, Andreas Hensel, Juergen J. Brandner, Kai zhang, Xiaoze Du, Yongping Yang

《化学科学与工程前沿（英文）》 2020年 第14卷 第3期   页码 350-364 doi: 10.1007/s11705-019-1894-0

摘要： Emulsion is a disperse system with two immiscible liquids, which demonstrates wide applications in diverse industries. Emulsification technology has advanced well with the development of microfluidic process. Compared to conventional methods, the microfluidics-based process can produce controllable droplet size and distribution. The droplet formation or breakup is the result of combined effects resulting from interfacial tension, viscous, and inertial forces as well as the forces generated due to hydrodynamic pressure and external stimuli. In the current study, typical microfluidic systems, including microchannel array, T-shape, flow-focusing, co-flowing, and membrane systems, are reviewed and the corresponding mechanisms, flow regimes, and main parameters are compared and summarized.

关键词： microfluidics     emulsification     capillary number     droplet breakup    

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A CFD study of the transport and fate of airborne droplets in a ventilated office: The role of droplet−droplet interactions

《环境科学与工程前沿（英文）》 2022年 第16卷 第3期 doi: 10.1007/s11783-021-1465-8

摘要：

• Coulomb and Lennard−Jones forces were considered for droplet interactions.

关键词： Droplet interactions     Aerosols     Colloids     CFD     Transport     Fate    

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Comparison of droplet distributions from fluidic and impact sprinklers

Xingye ZHU,Shouqi YUAN,Junping LIU,Xingfa LIU

《农业科学与工程前沿（英文）》 2015年 第2卷 第1期   页码 53-59 doi: 10.15302/J-FASE-2015049

摘要： To adapt to the trend toward low-energy precision irrigation, the droplet distributions for two new prototype sprinklers, outside signal sprinkler (OS) and fluidic sprinkler (FS), were compared with impact sprinkler (IS). A laser precipitation monitor was used to measure the droplet distributions. Droplet size and velocity distributions were tested under four operating pressures for nozzles 1.5 m above the ground. For the operating pressures tested, the mean OS, FS and IS droplet diameters ranged from 0 to 3.4, 0 to 3.5, 0 to 4.0 mm, respectively. The mean OS and FS droplet velocities ranged from 0 to 6.3 m·s , whereas IS ranged from 0 to 6.3 m·s . Being gas-liquid fluidic sprinklers, droplet distributions of the OS and FS were similar, although not identical. IS mostly produced a 0.5 mm larger droplet diameter and a 0.5 m·s greater velocity than OS and FS. A new empirical equation is proposed for determination of droplet size for OS and FS, which is sufficiently accurate and simple to use. Basic statistics for droplet size and velocity were performed on data obtained by the photographic methods. The mean droplet diameter (arithmetic, volumetric and median) decreased and the mean velocity increased in operating pressure for the three types of sprinkler.

关键词： outside signal sprinkler     fluidic sprinkler     impact sprinkler     sprinkler irrigation     droplet size     droplet velocity    

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Assessment and validation of liquid breakup models for high-pressure dense diesel sprays

Yi REN,Xianguo LI

《能源前沿（英文）》 2016年 第10卷 第2期   页码 164-175 doi: 10.1007/s11708-016-0407-9

摘要： Liquid breakup in fuel spray and atomization significantly affects the consequent mixture formation, combustion behavior, and emission formation processes in a direct injection diesel engine. In this paper, different models for liquid breakup processes in high-pressure dense diesel sprays and its impact on multi-dimensional diesel engine simulation have been evaluated against experimental observations, along with the influence of the liquid breakup models and the sensitivity of model parameters on diesel sprays and diesel engine simulations. It is found that the modified Kelvin-Helmholtz (KH)–Rayleigh-Taylor (RT) breakup model gives the most reasonable predicted results in both engine simulation and high-pressure diesel spray simulation. For the standard KH-RT model, the model constant for the breakup length has a significant effect on the predictability of the model, and a fixed value of the constant cannot provide a satisfactory result for different operation conditions. The Taylor-analogy-breakup (TAB) based models and the RT model do not provide reasonable predictions for the characteristics of high-pressure sprays and simulated engine performance and emissions.

关键词： breakup model     diesel engine     high-pressure injection     simulations    

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Analysis of the radiation heat transfer process of phase change for a liquid droplet radiator in space

Jinying YIN, Linhua LIU

《能源前沿（英文）》 2011年 第5卷 第2期   页码 166-173 doi: 10.1007/s11708-010-0105-y

摘要： The optimization of a space power system is greatly affected by the radiation heat transfer in a liquid droplet radiator (LDR). Radiation heat transfer in a two-dimensional bed of phase-change particle is modeled by solving the radiative transfer equation using the discrete ordinates method and the energy equation using the implicit finite difference method. The Mie theory is used to calculate the radiative properties of the droplet bed, whereas the effective medium theory is used to obtain the optical constants of partial solidification droplets. Multiple factors affect heat flux in the LDR, such as size distribution, flow velocity, phase change of droplets, layer thickness, droplet concentration in the layer, and material type of the work fluid; each of these must be analyzed. Calculations show that once size distribution is neglected, the relative error increases significantly. Size distribution has a remarkably strong effect on heat flux when the flow velocity of the working fluid is above 100 m/s. An increase in flow velocity leads to an increase in the total heat flux for the layer with a fixed volume fraction of droplets. The solidification zone occupies nearly half of the layer, and droplets of different sizes exhibit temperature differences to some extent due to local thermal non-equilibrium among them. Droplet concentration in the layer and the material type of the working fluid have strong effects on heat flux, whereas the thickness of the layer has a mild influence on heat flux.

关键词： radiation heat transfer     particle polydispersion     liquid droplet radiator     phase change    

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Modeling and simulation of droplet translocation and fission by electrowetting-on-dielectrics (EWOD)

Nathan HOWELL, Weihua LI

《机械工程前沿（英文）》 2010年 第5卷 第4期   页码 376-388 doi: 10.1007/s11465-010-0104-z

摘要： This paper discusses methods of microfluidic droplet actuation by means of electrowetting-on-dielectrics (EWOD) and provides a technique for modeling and simulating a microfluidic device by using the computational fluid dynamics (CFD) program, Flow3D. Digital or droplet microfluidics implies the manipulation of droplets on a scale of nanoliters (10 L) to femtoliters (10 L), as opposed to continuous microfluidics that involve the control of continuous fluid within a channel. The two operations in focus here are droplet translocation (moving) and droplet fission (splitting), in which the pressures and velocities within the droplet are analyzed and compared to existing works, both theoretical and experimental. The variation in the pressure of the leading and trailing faces of a droplet indicates the variation in surface energy—an important parameter that explains how a droplet will move toward a region of higher electric potential. The higher voltage on one side of a droplet reduces surface energy, which leads to an induced pressure drop, thus resulting in fluid motion. Flow3D simulations are for both water and blood droplets at voltages between 50 V and 200 V, and the droplet size, surface properties (Teflon coated), and geometry of the system are kept constant for each operation. Some peculiarities of the simulation are brought to light, such as instabilities of the system to higher voltages and fluids with higher dielectric constants, as well as the creation of a tertiary droplet when the applied voltage causes a large enough force during fission. The force distribution across the droplet provides a general understanding of the electrowetting effect and more specifically allows for a comparison between the effects that different voltages have on the forces at the droplet surface. The droplet position and mean kinetic energy of the droplet are also investigated and compared to other works, proving the dynamics of a droplet motion found here.

关键词： electrowetting-on-dielectrics (EWOD)     electrowetting     microfluidics     droplet translocation     droplet fission     Flow3D     dielectric constant    

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Dynamical analysis of droplet impact spreading on solid substrate

Zhaomiao LIU, Huamin LIU, Xin LIU,

《机械工程前沿（英文）》 2010年 第5卷 第3期   页码 308-315 doi: 10.1007/s11465-010-0020-2

摘要： This paper investigates the impact spreading of a droplet on a solid substrate using numerical simulation on the basis of a volume-of-fluid (VOF) model. The process of droplet spreading is described, the analysis of low speed and high speed droplet spreading, and more than one droplet spreading simultaneously is performed. The pressure, velocity, and spreading factor during the droplet spreading are reported. According to the spreading factor’s evolvement, the process of droplet spreading can be classified into spreading phase and recoiling phase. The spreading factors are almost the same at the low speed droplet spreading; however, the pressures on the substrate are quite different and air entrainment may be found as the impact speeds in a certain range. The impact speed impacts on the spreading factors in high speed droplet spreading. The spreading factor obviously increases with increasing impact speed; however, splashing will appear in the status when the speed is high enough in the high speed droplet spreading. The distance between the neighbor droplets affects the film’s quality, and only the distance between the static diameter and the maximum diameter can ensure the film’s quality. The results could help in understanding the process of droplet spreading and provide advice on the operation of a spray coating process.

关键词： droplet     impact spreading     numerical simulation    

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Synthesis of crystals and particles by crystallization and polymerization in droplet-based microfluidic

Jingtao WANG, Jin ZHANG, Junjie HAN,

《化学科学与工程前沿（英文）》 2010年 第4卷 第1期   页码 26-36 doi: 10.1007/s11705-009-0292-4

摘要： The recent advances in crystallization and polymerization assisted by droplet-based microfluidics to synthesize micro-particles and micro-crystals are reviewed in this paper. Droplet-based microfluidic devices are powerful tools to execute some precise controls and operations on the flow inside microchannels by adjusting fluid dynamics parameters to produce monodisperse emulsions or multiple-emulsions of various materials. Major features of this technique are producing particles of monodispersity to control the shape of particles in a new level, and to generate droplets of diverse materials including aqueous solutions, gels and polymers. Numerous microfluidic devices have been employed to generate monodisperse droplets of range from nm to μm, such as T junctions, flow-focusing devices and co-flow or cross-flow capillaries. These discrete, independently controllable droplets are ideal microreactors to be manipulated in the channels to synthesize the nanocrystals, protein crystals, polymer particles and microcapsules. The generated monodisperse particles or crystals are to meet different technical demands in many fields, such as crystal engineering, encapsulation and drug delivery systems. Microfluidic devices are promising tools in the synthesis of micron polymer particles that have diverse applications such as the photonic materials, ion-exchange and chromatography columns, and field-responsive rheological fluids. Processes assisted by microfluidic devices are able to produce the polymer particles (including Janus particles) with precise control over their sizes, size distribution, morphology and compositions. The technology of microfluidics has also been employed to generate core-shell microcapsules and solid microgels with precise controlled sizes and inner structures. The chosen “smart” materials are sensitive to an external stimulus such as the change of the pH, electric field and temperature. These complex particles are also able to be functionalized by encapsulating nanoparticles of special functions and by attaching some special groups like targeting ligands. The nucleation kinetics of some crystals like KNO was investigated in different microfluidic devices. Because of the elimination of the interactions among crystallites in bulk systems, using independent droplets may help to measure the nucleation rate more accurately. In structural biology, the droplets produced in microfluidic devices provide ideal platforms for protein crystallization on the nanoliter scale. Therefore, they become one of the promising tools to screen the optimal conditions of protein crystallization.

关键词： core-shell     monodisperse     nucleation     Microfluidic     different technical    

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Numerical study of droplet dynamics impinging onto steel plate covered with scale layer

Jan BOHá?EK, Ale? HORáK

《机械工程前沿（英文）》 2010年 第5卷 第4期   页码 389-398 doi: 10.1007/s11465-010-0108-8

摘要： The steel hot rolling process is inseparably connected to an oxide layer called “scale” at high temperatures. Hydraulic descaling of rolled material is a part of all rolling trains. Surface quality after descaling is fundamental for the final surface quality of a rolled product. The process itself is not theoretically well described; various different approaches have been used to clarify the descaling problem. This paper describes the dynamics of high-speed impact between the compressible water droplet and the steel scale layer. The phenomenon is known as water hammer effect. The purpose of this study is to numerically verify the fact that impact stress can be a significant factor during the descaling process. Considering a high droplet impact speed (100–300 ms ), inferential extremely short time interval (0.1–5 μs) peaks in impact pressure reaching 300 MPa can be found. Droplet dynamics was simulated with the help of LS-Dyna solver, whereas the stress analysis was performed in ANSYS interface. The extreme pressure peaks of very short duration in an impact area are a new phenomenon in the descaling theory.

关键词： hydraulic descaling     scale     rolling     water-hammer     descaling theory    

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Effect of UAV prewetting application during the flowering period of cotton on pesticide droplet deposition

Weixiang YAO, Xianju WANG, Yubin LAN, Ji JIN

《农业科学与工程前沿（英文）》 2018年 第5卷 第4期   页码 455-461 doi: 10.15302/J-FASE-2018232

摘要：

Prewetting process can reduce the contact angle between the droplet and the leaf blade, so that the droplet can more easily wet and spread, thereby increasing the quantity of deposition. To improve the effectiveness of pesticides on cotton leaves, prewetting by single-rotor electric unmanned aerial vehicles (UAV) was studied, focusing on the effects of pesticide deposition on cotton leaves during the flowering period. Cotton leaves in 0°–30°, 30°–60°, 60°–90° leaf blade angle ranges (angle between the leaf blade and the horizontal plane) were examined. In the first experiment, four different prewetting volumes (0, 1.6, 3.2 and 4.8 L) were sprayed by a single-rotor electric UAV on four cotton plots (plots A to D) each with an area of 120 m , and then each area was sprayed with a 0.8% (w/v) ponceau 2R solution by another single-rotor electric UAV. The results revealed that with no prewetting, droplet deposition quantity decreased with increasing leaf blade inclination. After prewetting, the mean droplet deposition quantity on plots B, C and D increased by 39.8%, 9.7% and 24.9%, respectively. The prewetting rate of 1.6 L per 120 m had the most significant effect on improving the deposition of droplets. It was also found that the mean droplet deposition quantity in each leaf blade angle range increased after prewetting. For the leaf blade angle range 60° to 90°, this increase was the most pronounced, with 0.043, 0.062, 0.057 and 0.048 L·cm in plots A–D, respectively. Also, droplet deposition uniformity in the leaf blade angle range 60°–90° was better after prewetting. These results should provide a valuable reference for future research and practice to improve the effectiveness of pesticides applied to cotton by aerial applications.

关键词： aerial spray     cotton     deposition     flowering period     leaf angle     prewetting     UAV    

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Droplet spectra and high-speed wind tunnel evaluation of air induction nozzles

Qing TANG, Liping CHEN, Ruirui ZHANG, Min XU, Gang XU, Tongchuan YI, Bin ZHANG

《农业科学与工程前沿（英文）》 2018年 第5卷 第4期   页码 442-454 doi: 10.15302/J-FASE-2017169

摘要：

A series of air induction nozzles were tested in a high-speed wind tunnel. Droplet size spectra were measured for four air induction nozzles (IDK-120-01, IDK-120-02, IDK-120-03 and IDK-120-04) each at three spray pressures (0.3, 0.4 and 0.5 MPa) and seven different air velocities (121.7, 153.4, 185.5, 218.4, 253.5, 277.5 and 305.5 km·h ). The measurement distance (0.15, 0.25 and 0.35 m) from the nozzle orifice was found to be important for the atomization of the droplets. The response surface method was used to analyze the experimental data. The results indicated that v and v of the droplets decreased quasi-linearly with increased wind speed, while v was affected by the quadratic of wind speed. v , v and v of the droplets were all proportional to the orifice size, and were not markedly influenced by the spray pressure. The percentage of the spray volume consisting of droplets with a diameter below 100 mm (%<100 mm) was found to be quadratically related to wind speed, and was not markedly influenced by the spray pressure and orifice size. However, the effect of the orifice size on the %<200 mm could not be ignored.

关键词： air induction nozzle     wind tunnel     aerial spray     droplet size spectra    

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Influence of sprinkler irrigation droplet diameter, application intensity and specific power on flower

Yisheng ZHANG, Delan ZHU

《农业科学与工程前沿（英文）》 2017年 第4卷 第2期   页码 165-171 doi: 10.15302/J-FASE-2017145

摘要： To determine the main parameters of droplet strike damage and avoid flower injury due to the unsuitable practices during sprinkler irrigation, an indoor experiment of irrigation droplet impact on cyclamen was conducted. The influences of different parameters such as droplet diameter, application intensity, specific power on flower strike damage was analyzed using Image Pro-Plus software to compute strike damage area and define damage level by sense-analysis. The results showed that a damage area of <1% represents a safe irrigation level, 1%–3% slight damage level, 3%–6% moderate damage level, and>6% heavy damage level. Equations of application intensity, specific power with sprinkler irrigation time and flower injury ratio were regressed against parameters which cause impact damages. The results indicated that specific power has a significant correlation with injury, and flower damage area increased as the increasing of the value of specific power for the same irrigation time. Application intensity was also correlated with injury when the droplet diameter was larger than 1 mm. When the duration of sprinkler irrigation was 1, 5 and 10 min, the threshold of impinging damage of application intensity was 25.30, 5.01 and 1.64 mm·h and the specific power was 0.467×10 , 9.340×10 and 3.110×10 W·m . These results provide a reference for determining the suitable values of sprinkler properties in operation design.

关键词： application intensity     damage     floriculture     flowers     specific power     sprinkler irrigation    

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Digital microfluidics: A promising technique for biochemical applications

He WANG, Liguo CHEN, Lining SUN

《机械工程前沿（英文）》 2017年 第12卷 第4期   页码 510-525 doi: 10.1007/s11465-017-0460-z

摘要：

Digital microfluidics (DMF) is a versatile microfluidics technology that has significant application potential in the areas of automation and miniaturization. In DMF, discrete droplets containing samples and reagents are controlled to implement a series of operations via electrowetting-on-dielectric. This process works by applying electrical potentials to an array of electrodes coated with a hydrophobic dielectric layer. Unlike microchannels, DMF facilitates precise control over multiple reaction processes without using complex pump, microvalve, and tubing networks. DMF also presents other distinct features, such as portability, less sample consumption, shorter chemical reaction time, flexibility, and easier combination with other technology types. Due to its unique advantages, DMF has been applied to a broad range of fields (e.g., chemistry, biology, medicine, and environment). This study reviews the basic principles of droplet actuation, configuration design, and fabrication of the DMF device, as well as discusses the latest progress in DMF from the biochemistry perspective.

关键词： digital microfluidics     electrowetting on dielectric     discrete droplet     biochemistry    

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细水雾与热烟气相互作用数值模拟研究

叶栋,蒋勇

《中国工程科学》 2007年 第9卷 第2期   页码 84-89

摘要：

使用CFD软件Fluent对火灾中热烟气与细水雾的相互作用过程进行了数值模拟研究。比较了灭火过 程中不同粒径细水雾在流场中的运动及其对灭火效果的影响，并研究了细水雾对着火房间火焰辐射的散射作用 及细水雾的聚合破碎过程对灭火效果的影响。模拟结果表明辐射是火灾中主要的热传递过程，粒径较大的水雾 比较容易离开回流区到达燃烧反应区。房间细水雾的通过吸收和散射作用减弱辐射强度，水雾在喷射初期可能 使燃烧速率增大，这些结果与实验事实相符

关键词： 细水雾     Fluent     热辐射     散射     聚合     破碎    

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Simulation of bubble column reactors using CFD coupled with a population balance model

Tiefeng WANG

《化学科学与工程前沿（英文）》 2011年 第5卷 第2期   页码 162-172 doi: 10.1007/s11705-009-0267-5

摘要： Bubble columns are widely used in chemical and biochemical processes due to their excellent mass and heat transfer characteristics and simple construction. However, their fundamental hydrodynamic behaviors, which are essential for reactor scale-up and design, are still not fully understood. To develop design tools for engineering purposes, much research has been carried out in the area of computational fluid dynamics (CFD) modeling and simulation of gas-liquid flows. Due to the importance of the bubble behavior, the bubble size distribution must be considered in the CFD models. The population balance model (PBM) is an effective approach to predict the bubble size distribution, and great efforts have been made in recent years to couple the PBM into CFD simulations. This article gives a selective review of the modeling and simulation of bubble column reactors using CFD coupled with PBM. Bubble breakup and coalescence models due to different mechanisms are discussed. It is shown that the CFD-PBM coupled model with proper bubble breakup and coalescence models and interphase force formulations has the ability of predicting the complex hydrodynamics in different flow regimes and, thus, provides a unified description of both the homogeneous and heterogeneous regimes. Further study is needed to improve the models of bubble coalescence and breakup, turbulence modification in high gas holdup, and interphase forces of bubble swarms.

关键词： bubble column     computational fluid dynamics     bubble breakup and coalescence     population balance model     bubble size distribution    

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标题 作者 时间 类型 操作

A review on emulsification via microfluidic processes

Yichen Liu, Yongli Li, Andreas Hensel, Juergen J. Brandner, Kai zhang, Xiaoze Du, Yongping Yang

期刊论文

A CFD study of the transport and fate of airborne droplets in a ventilated office: The role of droplet−droplet interactions

期刊论文

Comparison of droplet distributions from fluidic and impact sprinklers

Xingye ZHU,Shouqi YUAN,Junping LIU,Xingfa LIU

期刊论文

Assessment and validation of liquid breakup models for high-pressure dense diesel sprays

Yi REN,Xianguo LI

期刊论文

Analysis of the radiation heat transfer process of phase change for a liquid droplet radiator in space

Jinying YIN, Linhua LIU

期刊论文

Modeling and simulation of droplet translocation and fission by electrowetting-on-dielectrics (EWOD)

Nathan HOWELL, Weihua LI

期刊论文

Dynamical analysis of droplet impact spreading on solid substrate

Zhaomiao LIU, Huamin LIU, Xin LIU,

期刊论文

Synthesis of crystals and particles by crystallization and polymerization in droplet-based microfluidic

Jingtao WANG, Jin ZHANG, Junjie HAN,

期刊论文

Numerical study of droplet dynamics impinging onto steel plate covered with scale layer

Jan BOHá?EK, Ale? HORáK

期刊论文

Effect of UAV prewetting application during the flowering period of cotton on pesticide droplet deposition

Weixiang YAO, Xianju WANG, Yubin LAN, Ji JIN

期刊论文

Droplet spectra and high-speed wind tunnel evaluation of air induction nozzles

Qing TANG, Liping CHEN, Ruirui ZHANG, Min XU, Gang XU, Tongchuan YI, Bin ZHANG

期刊论文

Influence of sprinkler irrigation droplet diameter, application intensity and specific power on flower

Yisheng ZHANG, Delan ZHU

期刊论文

Digital microfluidics: A promising technique for biochemical applications

He WANG, Liguo CHEN, Lining SUN

期刊论文

细水雾与热烟气相互作用数值模拟研究

叶栋,蒋勇

期刊论文

Simulation of bubble column reactors using CFD coupled with a population balance model

Tiefeng WANG

期刊论文